Controlled electropolymerisation of a carbazole-functionalised iron porphyrin electrocatalyst for CO2 reduction

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Xin-Ming Hu, Zakaria Salmi, Mie Lillethorup, Emil B. Pedersen, Marc Robert, Steen U. Pedersen, Troels Skrydstrup and Kim Daasbjerg

doi.org/10.1039/C6CC00982D

Using a one-step electropolymerisation procedure, CO2 absorbing microporous carbazole-functionalised films of iron porphyrins are prepared in a controlled manner. The electrocatalytic reduction of CO2 for these films is investigated to elucidate their efficiency and the origin of their ultimate degradation.

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